phys.stat.sol.(b)209,485(1998)Subjectclassification:78.35.+c;S7.13
485
AnalyticalCalculationofStimulatedBrillouinScatteringinMagneticFieldsAppliedton-InSb1
K.L.Jat
DepartmentofPhysics,GovernmentDegreeCollege,Manasa-458110(M.P.),India(ReceivedJuly3,1998)
Forthestudyofparametricexcitation,wehaveconsideredthattheoriginofStimulatedBrillouinScattering(SBS)nonlinearinteractionliesinthethird-orderopticalsusceptibilityinacentrosym-metric,dopedsemiconductorwhichissubjectedtotransversemagneticfield.Thethird-orderopti-calpolarizationinaSBSsystemarisesduetononlinearcurrentdensityandacousto-opticalstrainofthemedium.ThedisplacementoflatticemotionandthresholdexpressionsaredeterminedandconditionsfortheonsetoftheSBSareobtained.Theinducedacousto-opticalpolarizationandeffectiveBrillouinpolarizationaredeterminedusingacoupledmodescheme.UsingtheeffectiveBrillouinpolarizationsoachieved,thetransmittedintensityandefficiencyoftheBrillouincellhavealsobeencalculated.Theeffectofwavenumber,electricfield,dopingandmagneticfieldondiffer-entparametersisalsostudiedandnumericalestimationsaremadeforn-InSbat77Kdulyshinedbyapulsed10.6mmCO2laser.Thelatticedisplacementissignificantlyenhancedbywavevector,electricfieldandtransversemagnetostaticfield.Itisobservedthattheacousto-opticalpolarizationincreaseswithmagneticfieldwhilethenonlinearinducedpolarizationdecreases.TheeffectiveBril-louinpolarizationincreaseswithwavenumber,electricfieldamplitudeandmagneticfieldwhichisrequiredtoachieveanoptical-phase-conjugationprocess.
1.Introduction
Nonlinearopticsdevelopedintoasignificantsubfieldofphysics.Itwasopenedupbytheadventoflaserwithhighpeakpowers.Theavailabilityoftunabledyelasershasmadedetailednonlinearspectroscopicstudiespossiblethroughoutthevisibleregionofthespectrumfrom0.35to0.9nm.Conversely,nonlineartechniqueshaveextendedtherangeoftunablecoherentradiationharmonicgeneration,parametricdownconversionandstimulatedBrillouinandRamanscatteringindifferentorders.Nonlinearopticalprocessesareessentialinmanyapplications.Modulatorsanddemodulatorsareusedinopticalcommunicationsystems.Saturationandgain(orexcitationofparameters)playanessentialroleinobtainingultrashortpulses.Thedomainoftime-resolvedmeasure-mentsmaybeextendedtothefemtoseconddomain.Thisopensupnewpossibilitiesinmaterialscienceandchemicalkinetics.Thefieldofnonlinearspectroscopyhasmaturedrapidlybutstillhasmuchpotentialforfurtherexplorationandexploitation.Theappli-cationsinchemistry,biology,medicine,materialstechnologyandspeciallyinthefieldofcommunicationsandinformationprocessingarenumerous,seee.g.[1].
ThestudyofStimulatedBrillouinScattering(SBS)insolidshasbeenanactiveareaofresearchduetoitsmanifoldtechnologicalapplicationsinthefieldofquantumelec-WorkdoneundertheUGC(Bhopal)minorresearchprojectªNonlinearOpticalSusceptibilityCalculationsinSemiconductorPlasmaº.
1
486K.L.Jat
tronicsandacousticspectroscopy.TheSBSmechanismshavebeenemployedinhighpowerlasersystemsforimprovementsinamplifiers,isolators,prepulsesuppression,en-ergyextraction,pulsecompressionetc.[2to5].SBSisalsoregardedasoneofthemosteffectivenonlinearopticalphenomenaresponsiblefortheoccurrenceofnonlinearopti-calphaseconjugation(NOPC),duetoitspurityandhighconversionefficiency[6].Recently,ithasbeenobservedthatinadopedcentrosymmetricsemiconductorcrystalthetransversemagneticfieldisfoundtoreducethethresholdpumpfieldrequiredfortheoccurrenceofSBSinhighlydopingregimes[7].
InaSBSsystemitisalsoobservedthatthegainissignificantlyenhancedunderhighpowerpulsedexcitationbelowthedamagethresholdandundertheinfluenceofatrans-versemagnetostaticfieldwhenthecyclotronfrequencyislessthantheacousticwavefrequency[8].
Asfarastoourknowledgenoattempthasyetbeenmadetostudythelatticedispla-cement,Brillouinpolarization,acousto-opticalpolarizationandBrillouincelldesigninatransverselymagnetized,dopedsemiconductor.Inthefieldofnonlinearoptics,itisprovedthatthescatteringoflaserbeamfromsoundinadopedmagnetizedsemicon-ductor,affordsaconvenientmeansofcontrollingthefrequency,intensityanddirection-alityofanopticalbeamaswellastheamplificationprocess[9].Recently,JatandGhosh[10]reportedanalyticallythestudyofSBSphenomenaandtheconsequentam-plificationprocess.
Inthepresentinvestigation,thehydrodynamicalmodelofplasmasandcoupledmodetheoryhavebeenusedtostudyanalyticallytheSBSofanelectromagneticmodepropa-gationinamagnetoactivesemiconductorplasma.Itisassumedthatinann-typehighlydopedcentrosymmetricsemiconductorcrystal,thethird-orderopticalsusceptibilityori-ginatesfromthefiniteinducedcurrentdensity(cd)anacousto-optical(ao)polarization.Thecrystalissubjectedtoatransversemagneticfield,andtheeffectofdopingiscon-sideredwiththeplasmafrequencywpcoveringtheentireinfraredspectrum.Usingthecoupledmodetheoryofplasmas,thethresholdE0thconditionfortheonsetoftheBrillouininstabilityandeffectiveBrillouinpolarizationPeffBisdetermined.Thedis-placementoflatticemotion(u)andtheelectronfluidvelocitiesintheCBband(v0xmdv0yoftheBrillouincellhavealsobeenstudiedinthepresenceofpumpandmagneto-staticfields.Thetheoryisbasedontheparametricexcitationsorcouplingofthreefinitewavesandthetimevaryingfieldwhichgivesrisetoacousto-opticalstrain,whichinturncandrivetheacousticwavesinthemedia.
2.TheoreticalFormulation
ForstudyingtheparametricexcitationoflaserbyBrillouinmodeinamagnetizeddopedsemiconductor,arisingduetothenonlineareffectiveopticalpolarization(Peff,thehydro-dynamicmodelofhomogeneous,one-component(electrononly),semiconductorplasmaofinfiniteextentisconsidered(i.e.kl(1Ykbeingthewavenumberofacousticmodeandlthemeanfreepathoftheelectrons).ThetheoreticalformulationstartswiththecalculationofthedisplacementoflatticemotionuandthetotalcurrentdensityJfortheresonantStokescomponentarisesduetononlinearinteractionofthewaves,followedbystudyingtheeffectiveBrillouinpolarizationPeffBthroughnonlinearpolarizationPcdarisingduetononlinearinducedcurrentandacousto-opticalstrainPao.Theentiretheoreticalanalysisisdividedintothefollowingthreesubsections.
StimulatedBrillouinScatteringinMagneticFieldsAppliedton-InSb
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2.1Totalinducedcurrentdensity
InordertocalculatethetotalinducedcurrentdensityJ,weapplythepumpelectricfieldE0exppk0xÀw0tparalleltotheacousticwavevectorka(alongthex-axis),andadcmagneticfieldB0,normaltok1alongthez-axis.Asthecrystalisassumedtobecentrosymetric,theeffectofanypseudo-potentialcanbeneglectedforanalyticalsimpli-city.Thenonlinearpolarizationarisingduetotheacousto-opticalstrainandthenon-linearinducedcurrentdensityisobtainedbyemployingthecoupledmodescheme.Thefollowingbasicequationsareemployedfortheanalysis:
d2uCd2udu
FsYÀ2Ga
dt2rdx2dtwhere
Fs
1d
eh2À1EeffÁE*1Y2rdx234561
dV0dV0e
EeffYV0nV0mdtdxdV1dV1e
E1V1ÂB0YnV1V0mdtdxdn1dn1dV0dV1
V0n1n00YdtdxdxdxPaoÀe0h2À1ru*ÁEeffYdE1n1eh2À1
Eeffr2u*Yee1dxwhere
EeffE0V0ÂB0X
Equation(1)representsthelatticemotioninthecrystal,risitsmassdensityandu
thelatticedisplacement,Gathephenomenologicaldampingparameteroftheacousticmode,Ctheelasticconstant,htherefractiveindexofthecrystal,ethedielectriccon-stantofthemediumandE1thespacechargeelectricfield.Equations(2)and(3)repre-sentthezerothandfirst-orderoscillatoryfluidvelocitiesofelectronswitheffectivemassmandchargee;nistheelectroncollisionfrequency.Ineq.(2),EeffrepresentstheeffectiveelectricfieldwhichincludestheLorentzforceV0ÂB0inthepresenceoftheexternalmagneticfieldB0.Equation(4)isthecontinuityequation,wheren0andn1aretheequilibriumandperturbedcarrierdensities,respectively.
Equation(5)showsthattheacousticwavegeneratedduetoacousto-opticalstrainmod-ulatesthedielectricconstantandgivesrisetoanonlinearinducedacousto-opticalpolari-zationPao.Ataveryhighfrequencyofthefieldafrequencywhichislargecomparedtothefrequenciesofmotionoftheelectronsinthemedium,thepolarizationofthemediumisconsideredneglectingtheinteractionofelectronswitheachotherandwiththeatomicnuclei.Equation(6)determinesthespacechargefieldE1,wheree1isthepermittivityofthecrystalathighfrequency.IntheaboveequationswehaveneglectedtheeffectduetoV0ÂB1byassumingthattheacousticwaveispropagatingalongthedirectionofthelong-itudinalelectricfield,inInSbifkistakenalong[011]andthelatticedisplacementalong[100].Theelectricfieldinducedbythewaveislongitudinal.
488K.L.Jat
Theacousto-opticforcegivesrisetoacarrierperturbationwithinthemediumwheretheBrillouinscatteringprocessisactive.Inadopedsemiconductor,thisdensitypertur-bationcanbeobtainedbyusingthestandardapproach[11].Differentiatingeq.(6)withrespecttotimeandusingeqs.(2)and(6),onegetsthefollowingsimplification:
d2n1dn1n0e222\"Y\"nnÀkhÀ1EeffxuÀikn1Ew1p
me1dt2dtwhere
2
\"2wpwp
7
w2
1À2c2Y
nwc
\"eE0wcV0yeEeffxYE
mminwhichEeffxE0V0B0x.Here,wceB0amisthecyclotronfrequencyand
wpn0e2ame0X5istheelectronplasmafrequencyofthemedium.WehaveneglectedtheDopplershiftundertheassumptionthatw0)n)kv0.WehaveconsideredthelowfrequencyperturbationstobeproportionaltoexpikaxÀwat,waYkacharacter-izingtheacousticwavepropagation,whileV0variesasexpÀiw0t.
Theperturbedelectronconcentrationn1willhavetwocomponentswhicharedistin-guishedasfastn1fandslown1scomponent,suchthatn1n1fn1s.Theslowcom-ponentisassociatedwiththelowfrequencyacousticwavewa,whilethefastcompo-nentoscillatesatthehighfrequencyelectromagneticwavew0Æwa.TakingonlytheStokescomponentofthescatteredelectromagneticwaveintoaccount,w1w0Æwaandk1k0ÀkaX
Forspatiallyuniformlaserirradiationjk0j%0yieldsjk1j%jkaj%jkj(say).
Weobtainthefollowingcoupledequationsfrom(7)underrotatingwaveapproxima-tion(RWA):
d2n1sdn1sdn*1f2\"\"nnÀEwp1s2dtdtdxand
d2n1fdn1fn0ek22dn*1s2\"*\"nnÀhÀ1EuÀEwX1feffpdt2dtme1dx8b8a
Itcanbeinferredfromeqs.(8a)and(8b)thattheslowandfastcomponentsofthe
densityperturbationsarecoupledtoeachotherviathepumpelectricfield.Thus,itisobviousthatthepresenceofthepumpfieldisthefundamentalnecessityforSBStooccur.
Fromequation(1)weobtainthedisplacementvector(u)oflatticemotionas
*eh2À1kw20jE0jjE1jjujY2jR*j2rw2Àwc0
where
220X5222
jR*jw2XaÀkVa4Gawa
9
Usingequations(8)and(9)weget
n0e0h2À12k2E*0ÁE1A*n1sY
2rR*10
StimulatedBrillouinScatteringinMagneticFieldsAppliedton-InSb
489
where
A
4
2
d21Àiw1nd2iwan1À
\"j2k2jE
5À1
Y
20X5222\"eamE0w2aw2Àw2Yd2w\"2E1cpÀw1,d2wpÀwa,Vacaristheacoustic00
velocityinthemedium.Fromtheaboveexpression,itisclearthatn1sdependsuponthemagnitudeofthepumpintensityIin,whereIin0X5he0c0jE0j2withc0theveloc-ityoflight.Thedensityperturbationsthusproducedaffectthepropagationcharacteris-ticsofthegeneratedwaves.
TheresonantStokescomponentofthecurrentdensityduetofinitenonlinearin-ducedpolarizationcanbegivenby
Jw1neeV1xn1seV0xY
fromtheaboveRWA,onegets
Jw1
iew2pw1E1
2w21Àwc
2222
iw2pee0khÀ1w0jE0jE1AX
2rR*w2Àw2c
0
11
12
Thefirsttermoftheaboveexpressionrepresentsthelinearcomponentofthein-ducedcurrentdensity.Thesecondtermrepresentsthenonlinearcouplingamongthe
threeinteractingwavesviathenonlinearcurrentdensity.Thecomponentsoftheoscil-latoryelectronfluidvelocityintheconductionbandofthecrystalinthepresenceofpumpandmagnetostaticfieldsareobtainedfromeq.(3)as
jV0xj
and
jV0yj
ewcjE0j
X2mw2Àwc0
13b
20X522mw20Àwcnw0
ew20jE0j
13a
2.2EffectiveBrillouinpolarization
Tobeginwith,letustreattheinducedpolarizationPcdw1asthetimeintegralofthe
currentdensityJw1
J
PcdJdtÀX14
iw1Usingeq.(12)andtheapproachofNeogiandGhosh[7],weobtainPcdduetotheperturbedcurrentdensity,
Pcd
2322\"2e2pw0khÀ1jE0jE10w
X22rjR*jw2Àw2w1c
0
15
Inobtainingeq.(15)wehaveomittedthefactorA,becausethevalueofitis
110À19%1inouranalysis.
NowitiswellknownthattheoriginoftheSBSprocessliesinthatcomponentofPcdwhichdependsonjE0j2E1.Thecorrespondingthird-ordersusceptibilityisknownasthe
490K.L.Jat
Brillouinsusceptibility.FromtheaboverelationwecandeterminethenatureofthethresholdfortheonsetofSBSsettingPcdw10,(i.e.A0).Thisconditionyields
2
mw2222221a40ÀwcjE0thjd2X1w1nd2wan2ekw0
16
Therefore,theinteractionbetweenthepumpandthecentrosymmetriccrystalwillbe
dominatedbytheSBSphenomenaatapumppowerlevelwellabovethethresholdfieldE0th.
BesidestheBrillouinpolarizationPcd,thesystemshouldalsopossesanacousto-opti-calpolarizationPao,arisingduetotheinteractionofthepumpwavewiththeacousticwavegeneratedinthemedium.
Thisisduetothefactthatthescatteringoflightfromtheacousticmodeaffordsaconvenientmeansofcontrollingthefrequency,intensity,anddirectionofanopticalbeam.Thistypeofcontrolmakespossiblealargenumberofapplicationsinvolvingthetransmission,displayandprocessingofinformation.Theacousto-opticalpolarizationisobtainedfrom(5)and(9)as
24222
e20khÀ1w0jE0jjE1jjPaojX
222rjR*jw2Àwc0
17
Fromeqs.(15)and(17)weobtaintheeffectiveBrillouinpolarizationbyusing
PeffBPcdPaoas
23
2222222\"wekw0hÀ1jE0jjE1jp
X18PeffB01
22ww2rjR*jw2Àw10c0
2.3EffectiveBrillouinsusceptibility,transmittedintensity
andefficiencyoftheBrillouincell
Inordertoinvestigatethethird-ordereffectiveBrillouinsusceptibility,weusethefol-lowingrelation:
ceffB
PeffB
X
e0jE0j2E1
19
SubstitutingthevaluesofPeffBfromeq.(18)ineq.(19),wecanobtainceffB.
UsingtheexpressionofPeffBdeducedforaninfinitemedium,onecancalculatetheelectricfieldamplitudeETinacrystalcelloflengthL[12],withtheassumptionthatthesamplelengthisabouttwoordersofmagnitudegreaterthanthepumpweave-length,
ETÀikLaejPeffBjX
20
Noweq.(20)canbeemployedtodeterminethetransmittedintensityITbyusingtherelations
IT1a2he0c0jETj2
as
ITk2L2jPeffBj2a2he0c0e2X
21
StimulatedBrillouinScatteringinMagneticFieldsAppliedton-InSb
491
TheefficiencyoftheBrillouincellb0isobtainbyb0ITaIias
b0Lae2k2ajE0j2jPeffBj2X
22
Eqs.(18),(19),(21)and(22)maybeusedtostudytheeffectiveBrillouinsusceptibility,transmittedintensityandefficiencyoftheBrillouincellmadeofacentrosymmetriccrystal.
3.ResultsandDiscussion
Inthepresentanalyticalinvestigation,thedisplacementoflatticemotion,effectivepolarization,transmittedintensityandefficiencyoftheBrillouincellarededucedinaheavilydopedmagnetizedsemiconductorcrystalduetononlinearcurrentdensityandacousto-opticalpolarizationprocess.Fornumericalappreciationthisanalysisisappliedtoaspecificcaseofacentrosymmetriccrystal,whichisassumedtobeirradiatedbya10.6mmCO2laser.
Itisawellknownfactthattheimportantpropertyattachedtothesolidstateplasmaisthatitretainsitsownphysicalpropertiesandyetattainstheplasmastateduetothepresenceoffreecarriersinsidethemedium.Theelasticpropertieswhicharerelatedtothedensityofthemediumdeterminethepropertiesofpropagation.Thefirstexperi-mentalobservationsofsoundwaveandotherpropertiesaremadeinInSbbyLibcha-berandVeilex[13].Thetheoryisalsoappliedton-InSbcrystalforanalyticalinvestiga-tion,becauseInSbisasingle-valleysemiconductorhavingalargedensityofmobileparticlesintheplasmacomparedtoothers,whileGaAsandSibotharemany-valley
Fig.1.Variationoflatticedisplace-mentuandthresholdelectricfieldE0thwithwavenumberkatwc1X6Â1014sÀ1
492
K.L.Jat
Fig.2.VariationofeffectiveBrillouinpolarizationPeffB(inmksunits)withwavenum-berkatE0107VmÀ1andwc1X6Â1014sÀ1
Fig.3.Variationofacousto-opticalpolarizationPaoandinducedpolarizationPcdwithwavenum-berskatE0107VmÀ1andwc1X6Â1014sÀ1
StimulatedBrillouinScatteringinMagneticFieldsAppliedton-InSb
493
semiconductors.ThebandgapofInSbisalsomatchedtothepulsewavelength10.6mmofCO2laser.
Thematerialandsystemconstantsaretakenas[14]:m0X015m0,wherem0isthefreeelectronmass,h3X9,r5X8Â103kgmÀ3,Ga2Â1010sÀ1,n3Â1011sÀ1,Va4X8Â103msÀ1,w01X78Â1014sÀ1,wa1012sÀ1,k05X92Â105mÀ1,ka2X08Â108mÀ1,andne2X44Â1024mÀ3,L10À4m,e115X8,e08X85Â10À12FCÀ1.Wenowfocusourattentiononthefactorsthataffectthedisplacementoflatticemotion.Variationoflatticedisplacement,polarizationandthresholdelectricfieldwithwavenum-ber,magneticandelectricfieldwasfound.Itwasfoundthatthethresholdelectricfielddecreaseswiththewavenumber(Fig.1),andthisisquiteobviousasthelower(lessthan4Â105mÀ1)thevalueofk,thegreaterwillbethedisplacement.Fig.1alsoshowsthatlatticedisplacementincreaseslinearlywithwavenumber.ThedependenceofeffectiveBril-louinpolarizationwithwavenumberisshowninFig.2.Itisseenthatthepolarizationincreasesparabolicallywithincreasingk.Fig3showsthevariationoftheacousto-opticalandinducedpolarizationwithwavenumberoftheincidentwave.Itisclearfromthefigurethat,asthewavenumberincreases,bothpolarizationsincreaseinaparabolicalform.Buttheorderofacousto-opticalpolarizationisalwayslargerthantheinducedpolarization.
Fig.4.Variationoflatticedis-placementuandeffectivepolarizationPeffBwithelec-tricfieldE0atk105mÀ1andwc1X6Â1014sÀ1
494K.L.Jat
Fig.5.Variationofacousto-opti-calpolarizationPaoandin-ducedpolarizationPcdwithelectricfieldE0atk105mÀ1andwc1X6Â1014sÀ1
TheeffectofelectricfieldamplitudeonlatticedisplacementandeffectiveBrillouinpolarizationcanbeobservedfromFig.4.Thedisplacementandpolarizationbothin-creaselinearlywiththeamplitudeofelectricfield.Thus,wemayconcludethatahighervalueofthefieldismoresuitableforSBSandamplificationofthescatteredsignal.Fig.5displaysthedependenceofacousto-opticalpolarizationandinducedpolarizationonelectricfield.BothtypesofpolarizationsintheSBSsystemincreaselinearlywiththeamplitudeofelectricfield
Fig.6to8depicttheinfluenceofmagneticfieldonthelatticedisplacement,effec-tivepolarizationandthresholdelectricfield.Fig.6illustratesthevariationoflatticedisplacementuandthresholdelectricfieldE0thwithmagneticfieldintermsofcyclotronfrequencyatfixedwavenumber.Itisfoundthatuisindependentatlowervaluesofmagneticfield,butitincreasesrapidlyathighervalues(largerthan1014).Itcanbeseenfromthefigurethatthethresholdelectricfielddecreaseswithmagneticfield.
ItisobservedfromFig.7thattheacousto-opticalpolarizationPaoincreaseswithmagneticfield,whiletheinducedpolarizationPcddecreases.Paobecomesmaximumatwc1X6Â1014sÀ1,butPcdgoestominimumatthisvalue.Fig.8showsthattheeffectiveBrillouinpolarizationchangesparabolicallywithincreasingmagneticfield.Thus,thresholdelectricfielddecreasesandlatticedisplacementandeffectivepolariza-tionincrease,sothatahighermagneticfieldwc w0issuitabletoobtaintheSBSprocessforamplificationphenomena.
StimulatedBrillouinScatteringinMagneticFieldsAppliedton-InSb
495
Fig.6.VariationoflatticedisplacementuandthresholdelectricfieldE0thwithmagnetostaticfieldintermsofcyclotronfrequencywcatk105mÀ1andE0107VmÀ1
Acloselookateqs.(19),(21),(22)andFigs.2,4and8revealsthattheeffectiveBrillouinsusceptibilityceffBorgain,transmittedintensityITandBrillouincelleffi-ciencyofacrystalincreasewithwavenumber,electricfieldamplitudeandmagneticfield,respectively.
TheabovediscussionsandanalysisrevealsthatlargeBrillouingain(orsuscept-ibilityorpolarizationorlatticedisplacement)andcellefficiencycanbeeasilyachievedinmagnetizedcentrosymmetriccrystalsbyselectingpropervaluesofdependingparameters.Thus,thepresenttheoreticalworkprovidesamodelmostappropriateforthefinitelaboratorysolidstateplasmaandfortheconstructionoftheBrillouincellanddiagnosticoflatticemotionandpolarizationofsemicon-ductors.
496
K.L.Jat
Fig.7.Variationofacousto-opticalpolarizationPaoandinducedpolarizationPcdwithmagneticfieldintermsofcyclotronfrequencywcatk105mÀ1andE0107VmÀ1
Fig.8.VariationofeffectiveBrillouinpolarizationwithmagneticfieldintermscyclo-tronfrequencywcat
5À17À1
k10mandE010Vm
StimulatedBrillouinScatteringinMagneticFieldsAppliedton-InSb
497
AcknowlegementTheauthoracknowledgesthefinancialsupportfromUGC,Bhopal(M.P.)underaminorresearchproject(1997).
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